Abstract
The mechanism of the reactions taking place in a photoredox system which exhibits extremely long lifetimes of redox products was investigated using photochemical, electrochemical, and radiation chemical methods. The system contains a tris(2,2'-bipyridine)ruthenium(II) derivative anchored to a positive poly-3,3-ionene polyelectrolyte (P3,3-Ru(bpy) 3 2+ ) as a photosensitiser 4-methoxy-N,N-dimethylaniline (4-MeODMA) as a quencher and a N,N,N',N'-tetramethyl-p-phenylenediamine derivative covalently bound to another poly-3,3-ionene polyelectrolyte (P3,3-TMPD) as a secondary donor
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