Abstract
AbstractMn(II)‐catalyzed alkylations of methyl N‐heteroarenes was reported via borrowing hydrogen strategy with alcohols as the alkylating reagent. The developed geometry‐constrained benzimidazole‐iminopyridyl ligand played a key role in promoting the transformation and stablizing the metal center. A wide range of alcohols (aromatic, heteroaromatic and aliphatic) and methyl N‐Heteroarenes could be able to apply in the current catalytic system, with TON up to 7400.
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