Abstract
Fluorescence analysis is one of the most popular methods in metal ions detection, but the background interference is an unavoidable obstacle in the fluorescence analysis of complex samples. In this work, a persistent luminescence nanoprobe was designed to detect iron ions in real samples by avoiding background interference. First, the Sr4Al14O25:Eu2+, Dy3+ persistent luminescent nanoparticles (PLNPs) were prepared by solid-state reaction protocols and polydopamine (PDA) encapsulation. After modification, these PLNPs@PDA showed better afterglow performance. More importantly, the PLNPs@PDA are highly selective toward iron ions, and could serve as an afterglow “turn off” nanoprobe for selective detection of iron ions through a dynamic quenching mechanism, with a detection limit of 2.86 μM. To further realize rapid and on-site detection, a test strip based on PLNPs@PDA was prepared and applied, which also showed good detection performance in real water samples. Compared with other detection methods, this afterglow imaging detection does not depend on expensive instruments, and can effectively shield the interference of background fluorescence from complex water samples, which has a good application prospects in the actual water sample. This work opens a new avenue for developing afterglow probe for the detection of metal ion in water samples without background interference.
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