Abstract
Dusty cirrus clouds, a rare phenomenon occurring approximately a few times a year globally, are associated with desert dust plumes in the upper troposphere. The formation of these clouds involves a high-humidity layer above a mineral dust-rich layer. In the intermediate layer between these two layers, initially, a thin cirrus cloud forms heterogeneously on the mineral dust particles. The latent heat release caused by the ice nucleation and radiative cooling above the thin cirrus cloud layer cause instability and convection to occur. This convection uplifts mineral dust particles even higher until the humid layer is fully mixed with the mineral dust, resulting in the dusty cirrus covering the humid layer.The objective of this study is to investigate the formation mechanisms of dusty cirrus clouds. Addressing the challenges highlighted by Seifert et al. (2023), current atmospheric models struggle to predict these events. This work aims to validate the hypothesis presented by Seifert and further advance the understanding of the formation mechanisms. The study involves a simulation study conducted using the UCLALES-SALSA large-eddy model (Tonttila et al., 2017). A case study is performed using the atmospheric conditions present during Saharan dust plumes over Europe in recent years.The simulated dusty cirrus clouds show that the upward transport of the mineral dust is not as effective as in the regional model study by Seifert et al. (2023). This is because the mineral dust which gets uplifted initially sediments down back to the original mineral dust layer with the sedimenting ice crystals. Also, the predominant mechanism for the instabilization of the air in the initial stages of the cloud formation is the latent heat release caused by the ice nucleation and the growth of the ice crystals, rather than the radiative cooling suggested by Seifert et al. (2023).In the future, simulations will be conducted using idealized cases to comprehensively understand the most relevant mechanisms involved in the formation of dusty cirrus clouds.
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