Abstract

We report a nuclear magnetic resonance study of the Cu nuclei in the paramagnetic phase of Ca${}_{0.85}$Sr${}_{0.15}$CuO${}_{2}$. By measuring the temperature dependence of the magnetic and quadrupolar shift and of the spin-lattice relaxation rate, we have obtained the following major results. With decreasing temperature, Ca${}_{0.85}$Sr${}_{0.15}$CuO${}_{2}$ undergoes two successive crossovers: a dimensionality crossover from a two-dimensional to a three-dimensional (3D) Heisenberg antiferromagnet followed, very close to ${T}_{N},$ by a spin-degree crossover from a 3D Heisenberg to a 3D $\mathrm{XY}$ antiferromagnet. There is no evidence for any structural changes accompanying the magnetic phase transition. The values of the hyperfine coupling constants ${A}_{c},$ ${A}_{\mathrm{ab}},$ and $B$ have been determined.

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