Abstract

Chiral spin textures in ultrathin films, such as skyrmions or chiral domain walls, are believed to offer large performance advantages in the development of novel spintronics technologies. While in-plane magnetized films have been studied extensively as media for current- and field-driven domain wall dynamics with applications in memory or logic devices, the stabilization of chiral spin textures in in-plane magnetized films has remained rare. Here we report a phase of spin structures in an in-plane magnetized ultrathin film system where out-of-plane spin orientations within domain walls are stable. Moreover, while domain walls in in-plane films are generally expected to be non-chiral, we show that right-handed spin rotations are strongly favoured in this system, due to the presence of the interfacial Dzyaloshinskii–Moriya interaction. These results constitute a platform to explore unconventional spin dynamics and topological phenomena that may enable high-performance in-plane spin-orbitronics devices.

Highlights

  • Chiral spin textures in ultrathin films, such as skyrmions or chiral domain walls, are believed to offer large performance advantages in the development of novel spintronics technologies

  • In-plane magnetized films are a textbook case[1]: it is generally expected that ultrathin films have Neel wall textures where the spin vector rotates within the plane[2], and thicker films have Bloch wall textures where spins tilt through out-of-plane alignments[3,4]

  • Spinpolarized low-energy electron microscopy (SPLEEM)[19,20] was used to measure maps of the orientation of the magnetization vector in ultrathin, single-crystalline Fe/Ni bilayers grown on a W(110) crystal

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Summary

Introduction

Chiral spin textures in ultrathin films, such as skyrmions or chiral domain walls, are believed to offer large performance advantages in the development of novel spintronics technologies. While domain walls in in-plane films are generally expected to be non-chiral, we show that right-handed spin rotations are strongly favoured in this system, due to the presence of the interfacial Dzyaloshinskii–Moriya interaction. These results constitute a platform to explore unconventional spin dynamics and topological phenomena that may enable high-performance in-plane spin-orbitronics devices. Modelling the domain walls in Monte-Carlo simulations, we show that their stability can be understood by taking into account a uniaxial anisotropy contribution, a perpendicular anisotropy contribution as well as the contribution of the interfacial DMI

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