Abstract
Publisher Summary This chapter illustrates that Time-resolved Infrared spectroscopy (TRIR) has been highly successful for probing organometallic reactions in conventional solvents. The chapter shows that it is equally successful for probing such reactions in supercritical fluids, particularly scCO2. The combination of TRIR and scCO2 provides a unique approach to study the interaction of CO2 to metal centers and hence the co-ordination chemistry of CO2. With improved sensitivity of TRIR instrumentation the technique is no longer restricted to organometallic compounds and it has been successfully shown that it can be applied to short-lived organic species in conventional solvents.
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