Abstract

Positive transient optical gain has been demonstrated in Ho3+-doped transparent oxyfluoride glass-ceramics. A pump and probe experiment has been designed to show this result. High power laser pulses at 532nm were used as the pump source to strongly populate the Ho3+S25:F45 level due to nonresonant ground state absorption. Low power cw laser radiation at 750nm was used as the probe beam. The signal beam stimulates the emission associated with the Ho3+S25:F45→I75 electronic transition at 750nm. In addition to this, the high power pump pulses provide population inversion between the S25:F45 and I75, initial and final states of the transition, respectively, giving rise to the optical amplification of the signal beam. A gain coefficient of 3.7cm−1 (∼16dB∕cm) was obtained for a pump energy density of about 135mJ∕cm2 and a signal beam power density of 6μW∕cm2.

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