Abstract
An ultrasound-assisted three-component, one-pot domino reaction with ferrocenecarboxaldehyde is herein reported. The sequence of reactions entails the allylindation and dehydrative alkylation of stabilized C-nucleophiles (e.g. electron-rich – (hetero)aromatics and stabilized enols) and N-nucleophiles (e.g. azoles). Sonochemical reactions have been performed in three different high-intensity reactors: a bath (20.3kHz, 60W), as well as two cup horns working at 19.9kHz (75W) and 300.5kHz (70W) giving a library of 18 new ferrocenyl derivatives.
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