Abstract
The base strength and the nature of the counterions have important effects on the synthesis of tetrathiafulvalene (TTF) by base-induced isomerization of 1,4,5,8-tetrathianaphthalene (TTN). This kind of rearrangement is also applied to the synthesis of 1,4-dithiafulvenes from 1,4-dithiins. A new synthesis of TTN is also reported.
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