Observation and Classification of Low-Altitude Haze Aerosols Using Fluorescence–Raman–Mie Polarization Lidar in Beijing during Spring 2024

Abstract

Haze aerosols have a profound impact on air quality and pose serious health risks to the public. Due to its geographical location, Beijing experienced haze events in the spring of 2024. Lidar is an active remote sensing technology with a high spatiotemporal resolution and the ability to classify aerosols, and it is essential for effective haze monitoring. This study utilizes fluorescence–Raman–Mie polarization lidar with an emission wavelength of 355 nm, employing the δp-Gf method based on the particle depolarization ratio at 355 nm (δp355) and the fluorescence capacity (Gf), and combines meteorological data and backward-trajectory analysis to observe and classify low-altitude haze aerosols in Beijing during the spring of 2024. Notably, a mining dust event with strong fluorescence backscatter was detected. The haze aerosols were categorized into three types: pollution aerosols, desert dust, and mining dust. Their optical properties were summarized and compared. Desert dust showed a particle depolarization ratio range of 0.23–0.39 and a fluorescence capacity range from 0.18 × 10−4 to 0.63 × 10−4. Pollution aerosols had a larger fluorescence capacity but a lower depolarization ratio compared to desert dust, with a fluorescence capacity ranging from 0.55 × 10−4 to 1.10 × 10−4 and a depolarization ratio ranging from 0.10 to 0.17. Mining dust shared similar depolarization characteristics with desert dust but had a larger fluorescence capacity, ranging from 0.71 × 10−4 to 1.23 × 10−4, with a depolarization ratio range of 0.30–0.39. This study validates the effectiveness of the δp355-Gf method in classifying low-altitude haze aerosols in Beijing. Additionally, it offers a new perspective for more detailed dust classification using lidar. Furthermore, utilizing the δp355-Gf classification method and the δp355-Gf distributions of three typical aerosol samples, we developed a set of equations for the analysis of mixed aerosols. This method facilitates the separation and fraction analysis of aerosol components under various mixing scenarios. It enables the characterization of variations in the three types of haze aerosols at different altitudes and times, offering valuable insights into the interactions between desert dust, mining dust, and pollution aerosols in Beijing.