Numerical Simulation on the Production of Reactive Oxygen Species in Atmospheric Pulse-Modulated RF Discharges with He/O2 Mixtures

Abstract

By choosing an appropriate duty cycle and modulation frequency, the pulse-modulated RF discharge can be optimized to provide a high-density atmospheric plasma with a reduced power consumption but without the risk of gas heating in pure helium. In this paper, we presented a fluid model to investigate the generation of reactive oxygen species (ROS) in an atmospheric pulse-modulated RF discharge with He/O2 mixtures. The numerical results show that modulated by a pulse the electrons could not fully interact with the oxygen molecules, then leading to a less consumption of electrons. Thus, the production of ground state atomic oxygen, excited atomic oxygen and single delta oxygen (SDO) are suppressed, however, due to the reduced power dissipation under pulse modulation, the production of ground state atomic oxygen and excited atomic oxygen are still effective. Consequently, the duty cycle and modulation frequency can also be used to manipulate the generation of ROS in an atmospheric RF discharge.