Nuclear Data and the Effect of Gadolinium in the Moderator

Abstract

Recent cross-section measurements on gadolinium have raised concerns over the accuracy of moderator poison reactivity coefficient calculations. Measurements have been made at the ZED-2 (Zero Energy Deuterium) critical facility, Chalk River Laboratories, AECL, to study the reactivity effect of gadolinium in the moderator. Since the neutron capture cross-section of boron is well known, measurements were also made with boron to provide calibration data for measurements with gadolinium. The measurements have been used to quantify the bias of the reactivity effect in full-core simulations of ZED-2 using MCNP, a neutron transport code used extensively for simulations of nuclear systems, along with the ENDF/B-VII.0 cross-section data. The results showed a bias of -0.41 ± 0.07 mk/ ppm, or -2.1% ± 0.3%, given a reactivity worth of -20.1 mk/ppm for gadolinium. Additional simulations also show that the gadolinium neutron capture cross-section has been over-corrected, relative to previous evaluations, in a beta version of ENDF/B VII.1, which incorporates the Leinweber data.