Nonmonotonous atomic motions in metallic glasses

Abstract

Peculiar temporal intermittent microscopic dynamics has been recently reported during structural relaxation in metallic glasses, though its origin is poorly understood. By using x-ray photon correlation spectroscopy, we have investigated the atomic motions in a model system of metallic glass with distinct stability and in situ stress states. We find that the microscopic dynamics can be tuned from dramatically nonmonotonous to monotonous. The intermittent dynamics is always accompanied by the activation of a secondary relaxation process, as indicated by the drop of the initial nonergodic plateau of the intensity-intensity correlation function. Both phenomena depend on the material state and can be suppressed by simultaneously lowering the fictive temperature and external loading, leading the glass in a stationary metastable state which appears independent on the thermal history of the system.