Abstract
We report on pump-probe experiments on single molecules in a solid matrix, with strong laser fields and on a new host-guest system, dibenzanthanthrene in a naphthalene crystal. Besides strong light-shifts of the molecular lines, we observe the hyper-Raman resonance and for strong pump and probe beams, we also observe subharmonic resonances due to a ‘kicked pendulum’ motion of the Bloch vector. The experimental results are in very good agreement with calculations based on Bloch's equations, demonstrating their validity for single molecules in solids under intense resonant fields.
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
