Abstract
This review describes the magnetization-induced second harmonic generation (MSHG) in (FeIIxCrII1-x)1.5[CrIII(CN)6]·E 7.5H2O. The polarization of SH light of the (FeIIxCrII1-x) 1.5 [CrIII(CN)6]·7.5H2O films was rotated by an applied external magnetic field. The observed SH rotation angle of 1.3® was much larger than the Faraday rotation angle of 0.079® at 388 nm. This SH rotation is ascribed to the interaction between the electric polarization along the out-of-plane of film and spontaneous magnetization. The magnetic linear term (χijkLmagn(1))contributed particularly to the SH rotation.
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