Nonequilibrium electron distributions in a three-subband InGaAs/InAlAs quantum well studied via double resonance spectroscopy

Abstract

Midinfrared optical pumping of electrons from the ground (n=1) to the first excited (n=2) subband of the quantum well produces a strongly nonthermal electron distribution which is probed spectroscopically. Two sharp induced absorption peaks appear, associated with electrons which have scattered from the upper subband via longitudinal optical (LO) phonon emission and absorption. The presence of the phonon absorption channel evidences the importance of nonequilibrium LO phonon populations (nph∼1), and the impact on the nonradiative intersubband scattering rates in quantum cascade laser devices is explored.