Abstract

ABSTRACTThe systematic variations of experimentally determined exchange and hyperfine (h.f.) interactions between Eu2+ ions are compared firstly within the EuX (X=0,S,Se,Te) series of compounds and secondly in the magnetic dilution system EuxSr1−xS. Reasonably relations can be established between the individual nearest and next nearest neighbour exchange interactions (J1,J2 ) and the transferred h.f. interactions (ΔB1 , ΔB2 ), respectively, by considering their variations with the Eu–Eu distances (R1,R2). Using these results, the measured mean hyperfine field, BI(x), and the ferromagnetic saturation h.f. field, B↑↑ (x), of the EuxSr1−xS system can be related reasonably well to the ferro- and paramagnetic phase boundaries, Tc(x) and θ (x), respectively.

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