NEUTRON-RICH CHROMIUM ISOTOPE ANOMALIES IN SUPERNOVA NANOPARTICLES

Abstract

Neutron-rich isotopes with masses near that of iron are produced in type Ia and II supernovae. Traces of such nucleosynthesis are found in primitive meteorites in the form of variations in the isotopic abundance of 54Cr, the most neutron-rich stable isotope of chromium. The hosts of these isotopic anomalies must be presolar grains that condensed in the outflows of supernovae, offering the opportunity to study the nucleosynthesis of iron-peak nuclei in ways that complement spectroscopic observations and can inform models of stellar evolution. However, despite almost two decades of extensive search, the carrier of 54Cr anomalies is still unknown, presumably because it is fine-grained and is chemically labile. Here we identify in the primitive meteorite Orgueil the carrier of 54Cr-anomalies as nanoparticles, most likely spinels that show large enrichments in 54Cr relative to solar composition (54Cr/52Cr ratio >3.6xsolar). Such large enrichments in 54Cr can only be produced in supernovae. The mineralogy of the grains supports condensation in the O/Ne-O/C zones of a type II supernova, although a type Ia origin cannot be excluded. We suggest that planetary materials incorporated different amounts of these nanoparticles, possibly due to late injection by a nearby supernova that also delivered 26Al and 60Fe to the solar system. This idea explains why the relative abundance of 54Cr and other neutron-rich isotopes vary between planets and meteorites. We anticipate that future isotopic studies of the grains identified here will shed new light on the birth of the solar system and the conditions insupernovae.