Abstract

There has been much effort to provide eco-friendly and biodegradable materials for the next generation of composite products owing to global environmental concerns and increased awareness of renewable green resources. This review article uniquely highlights the use of green composites from natural fiber, particularly with regard to the development and characterization of chitosan, natural-fiber-reinforced chitosan biopolymer, chitosan blends, and chitosan nanocomposites. Natural fiber composites have a number of advantages such as durability, low cost, low weight, high specific strength, non-abrasiveness, equitably good mechanical properties, environmental friendliness, and biodegradability. Findings revealed that chitosan is a natural fiber that falls to the animal fiber category. As it has a biomaterial form, chitosan can be presented as hydrogels, sponges, film, and porous membrane. There are different processing methods in the preparation of chitosan composites such as solution and solvent casting, dipping and spray coating, freeze casting and drying, layer-by-layer preparation, and extrusion. It was also reported that the developed chitosan-based composites possess high thermal stability, as well as good chemical and physical properties. In these regards, chitosan-based “green” composites have wide applicability and potential in the industry of biomedicine, cosmetology, papermaking, wastewater treatment, agriculture, and pharmaceuticals.

Highlights

  • Nowadays, ecological concerns have resulted in renewed interest in natural materials

  • As a biomaterial form, chitosan can be made into a few forms, such as hydrogels, sponges, films which appear in 3D forms, and porous membrane which appears in 2D form, and each of them have specific applications in industries [75,76]

  • The good mixing of chitosan powder, acid, aceticin acid, and/or water followed by ultrasonic atomization–freeze casting andformic drying resulted excellent l-lactic acid in distilled by ultrasonic atomization–freeze casting and dryfiber formability, as well water as thefollowed minimization of volatile organic solvent use, which made ingobtained resultedchitosan in excellent fiber formability, as well as the minimization of volatile organic the nanofibers safe, environmentally friendly and compatible

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Summary

Introduction

Ecological concerns have resulted in renewed interest in natural materials. The need for more versatile polymer-based materials has led to increasing interest in polymer composites filled with natural, organic fillers, for example, fillers that are biodegradable and come from renewable sources [5,6,7,8]. Biomaterials are crucial in the development of a sustainable environment. Even though biomaterials are newly in development for the delivery of drugs, tissue engineering, and medical diagnostics, but there has been good improvement for both physical and chemical methods that can manage biological responses [9]. This review paper discusses green composites of natural fibers in detail and discusses the development and characterization of chitosan, natural-fiber-reinforced chitosan biopolymers, chitosan blends, as well as chitosan nanocomposites

Natural Fiber
Types of Green Composites and Chemical Composition of Natural Fibers
Mechanical Properties of Green Fibers
Advantages and Disadvantages of Chitosan
Chemical and Physical properties of Chitosan
Structure
Partially
References deacetylation
Thermal Properties of Chitosan
Dipping and Spray Coating
Freeze Casting and Drying
Layer-by-Layer
Extrusion
Mechanical
Thermal Properties of Chitosan-Based Green Composites
Chitosan-Blend Composites
Thermal Properties of Chitosan-Blend Composite
Mechanical Properties of Chitosan Hybrid Composites
Thermal Properties of Chitosan Hybrid Composites
Application of Chitosan-Based Green Composites
Drug Delivery
Wound Dressing
Food Packaging
Dermatology and Skin Care
Cosmetics for Oral Care Products
10. Challenges and Opportunities
Findings
11. Conclusions
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