Abstract

The development of a scalable and cost-effective nanofabrication method is of key importance for future advances in nanoelectronics. Thermal scanning probe lithography (t-SPL) is a growing nanopatterning method with potential for parallelization, offering unique capabilities that make it an attractive candidate for industrial nanomanufacturing. Here, we demonstrate the possibility to apply t-SPL for the fabrication of graphene devices. In particular, we use t-SPL to produce high performing graphene-based field effect transistors (FETs). The here described t-SPL process includes the fabrication of high-quality metal contacts, as well as patterning and etching of graphene to define the active region of the device. The electrical measurements on the t-SPL fabricated FETs indicate a symmetric conductance at the Dirac point and a low specific contact resistance without the use of any contact engineering strategy. The entire t-SPL nanofabrication process is performed without the need for masks, and in ambient conditions. Furthermore, thanks to the t-SPL in situ simultaneous patterning and imaging capability, no markers are required. These features substantially decrease fabrication time and cost.

Highlights

  • We report the application of thermal scanning probe lithography (t-SPL) performed in ambient conditions for the fabrication of graphene field-effect transistors (GFETs)

  • Monolayer graphene in both channel and contact regions is in direct contact with the t-SPL resist during all the lithographic steps

  • Without the use of contact engineering, we find that the GFETs fabricated using t-SPL exhibit a relatively low specific contact resistance of 600 Ω⋅μm

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Summary

Introduction

Novel nano-patterning techniques have been explored for fabricating nanoscale devices.[12,13,14,15] Among those, thermal scanning probe lithography (t-SPL) is an attractive choice for multiple reasons.[12,16,17,18,19,20] First, t-SPL is a maskless technique and is capable of patterning nanoscale features with sub-10 nm resolution.[17,21] Second, the entire t-SPL nano-patterning process can take place in atmospheric condition or N2, which is a considerable advantage for achieving a cost-effective nano-patterning process. The fabrication of graphene functional devices generally requires multiple patterning steps for defining the device active region and patterning metal contacts on graphene. More importantly, a recent study has demonstrated that t-SPL can pattern high-performing and low-resistance metal contacts on monolayer MoS2.24 the application of t-SPL for the fabrication of graphene devices remains largely unexplored.

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