Abstract

Electroactive hydrogels that exhibit large deformation in response to an electric field have received significant attention as a potential actuating material for soft actuators and artificial muscle. However, their mechanical actuation has been limited in simple bending or folding due to uniform electric field modulation. To implement complex movements, a pre-program, such as a hinge and a multilayer pattern, is usually required for the actuator in advance. Here, we propose a reprogrammable actuating method and sophisticated manipulation by using multipolar three-dimensional electric field modulation without pre-program. Through the multipolar spatial electric field modulator, which controls the polarity/intensity of the electric field in three-dimensions, complex three-dimensional (3D) actuation of single hydrogels are achieved. Also, air bubbles generated during operation in the conventional horizontal configuration are not an issue in the proposed new vertical configuration. We demonstrate soft robotic actuators, including basic bending mechanics in terms of controllability and reliability, and several 3D shapes having positive and negative curvature can easily be achieved in a single sheet, paving the way for continuously reconfigurable materials.

Highlights

  • Electroactive hydrogels that exhibit large deformation in response to an electric field have received significant attention as a potential actuating material for soft actuators and artificial muscle

  • As many previous studies in many research groups show, electroactive hydrogel, which reacts to the electric field, has a swell-deswell characteristic depending on the intensity or polarity of the electric field, which can be used to implement shape-morphing[1,25,30]

  • We have developed a technique to dynamically transform and reconfigure 2D hydrogel copolymer sheets into predictable and sophisticated 3D shapes not limited by pre-programmed patterns within the material

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Summary

Introduction

Electroactive hydrogels that exhibit large deformation in response to an electric field have received significant attention as a potential actuating material for soft actuators and artificial muscle Their mechanical actuation has been limited in simple bending or folding due to uniform electric field modulation. An electric field applied to a polyelectrolyte network locked in an electrolyte solution causes an asymmetrical dispersion of the ions, creating an osmotic pressure difference that was swelling and deforms the gel These physical and chemical processes are similar to the transfer ion exchange between the cell membrane and its environment[23,24].

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