Abstract

AbstractFluid systems in inverted rifted margins are challenging to interpret because fractures formed before compression were often reactivated acting as fluid pathways as new ones formed. Deciphering the fracture and fluid flow history in such complex settings has key implications for the prediction of the distribution of mineral resources. As an example, we reconstruct the fluid flow evolution of a portion of the inverted Pyrenean rift, the Upper Pedraforca thrust sheet, from the Mesozoic extension to the Alpine orogeny. We combine structural analysis and petrographic, geochemical and geochronological data obtained from 87 samples of fracture‐filling carbonate cements. During the Late Jurassic‐Early Cretaceous, low‐temperature seawater produced dolomitization of Jurassic and Lower Cretaceous limestones in an extensional setting. During the Early Cretaceous salt‐related extension, formation waters, probably evolved seawater or fluids that interacted with Triassic evaporites, at temperatures from 125 to 149°C migrated through fractures. The formation of breccias within post‐salt rocks in primary weld zones facilitated the upward migration of formation waters that interacted with pre‐salt rocks with high 87Sr/86Sr ratios. Formation waters at temperatures of 80°C migrated during the emplacement of the Upper Pedraforca thrust sheet in the Late Cretaceous‐Palaeocene. These fluids interacted with Upper Cretaceous Carbonates and/or Triassic evaporites. In contrast, the influence of meteoric fluids increased in shallower positions due to the exhumation of the SE Pyrenees during the Eocene‐Oligocene. Coevally, hot dolomitizing fluids migrated along diapir walls during the formation of secondary welds. Supergene ores documented in diapiric areas worldwide related to meteoric fluids, and the similar meteoric percolation occurred in the Upper Pedraforca thrust sheet, suggest that supergene mineralization could be found in the Pyrenees. Brecciation of rocks in primary weld zones and evaporite detachments, where mineralization accumulate in fractures from basement‐derived fluids, also suggests that similar ores could be found in the Pyrenees.

Highlights

  • Pre-­compressive thick evaporite units forming diapirs and/or detachment levels, can strongly control the palaeohydrology of fold and thrust belts and their related foreland basins, because fluids migrate induced by tectonic and topographic gradients in areas adjacent to evaporite bodies or along their boundaries (Crognier et al, 2018; Fischer et al, 2009, 2013; Moragas et al, 2020; Reuning et al, 2009; Smith et al, 2012)

  • The results of this study provide absolute time constraints and knowledge about: (1) how syn-t­ectonic fluid flow is recorded and distributed in sedimentary basins involved in long-­lasting deformation and (2) what the potential impact is of the changes in palaeofluid systems on the development and/or alteration of ore mineralization in diapir structures

  • | 29 unravelled from the combined study of fracture orientations, and petrographic, geochemical and geochronological analyses, leading to the following conclusions: 1. Mg-r­ ich low-­temperature seawater caused the dolomitization of thick Jurassic and Lower Cretaceous carbonate units at shallow burial conditions during Late Jurassic and Early Cretaceous extensional events

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Summary

Introduction

Pre-­compressive thick evaporite units forming diapirs and/or detachment levels, can strongly control the palaeohydrology of fold and thrust belts and their related foreland basins, because fluids migrate induced by tectonic and topographic gradients in areas adjacent to evaporite bodies or along their boundaries (Crognier et al, 2018; Fischer et al, 2009, 2013; Moragas et al, 2020; Reuning et al, 2009; Smith et al, 2012). Geological resources such as hydrocarbons, accumulate below evaporite seals and structural traps (e.g. folds and faults), which form due to salt and gypsum flow during rifting and thrusting (Allen & Allen, 2005; Davison et al, 2000). Other resources, such as metalliferous ore deposits (i.e. Pb-Z­ n), can be associated with the interaction of fluids with saline bodies (Perona et al, 2018; Rouvier et al, 1985; Sheppard et al, 1996). Considering the importance of salt-­related structures on the development and storage of resources of economic interest, the overarching aim of this study is to characterize the heterogeneity and evolution of fluid systems in sedimentary basins affected by rift-­related diapirism, as well as by subsequent inversion during orogenic compression

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