Abstract

Ionization yields are reported for Ar, Kr and Xe in ultrastrong fields from 1015 W cm−2 to 1018 W cm−2. Non-sequential ionization (NSI) is shown to be a robust and general feature in ultrahigh field ionization. NSI yields measured are consistent with the trends predicted by a rescattering model, but as one proceeds to higher Z atoms more NSI is observed than predicted theoretically. Additional recollision mechanisms that may need to be considered in future theories of ultrastrong field–atom interactions include ‘chain’ NSI, NSI from excited states of the atom (e.g. Rydberg states or inner-shell holes) and the possibility of ultrastrong field enhanced recollision/impact processes.

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