Abstract

Shear thickening fluids (STFs) have attracted increasing attention as smart materials with unique rheological properties. However, the preparation of STFs usually relies on a composite system of spherical nanoparticles with polyethylene glycol. In this work, novel multi-phase STFs (ILSTFs) were prepared in an ionic liquid by incorporating nanosized SiO2 and rod-shaped calcium metasilicate (CaSiO3) particles as a dispersed phase. Compared to traditional STFs, ILSTFs demonstrate excellent thermal stability. Rheological tests indicate that ILSTFs exhibit continuous shear thickening behavior, resulting in excellent energy absorption and impact wear resistance. In addition, ILSTFs can serve as a new type of lubricant. The tribological properties and impact resistance of ILSTFs were highly correlated with the shear thickening effect, with the multi-phase ILSTF system with CaSiO3 demonstrating superior impact wear resistance compared to the single-phase system. In this study, finite element analysis (FEA) is further utilized to investigate the local damage evolution and energy absorption rate of STF under impact loading, providing insights into the underlying mechanism. This ionic liquid-based STF holds promise for applications as a flexible filling component in the fields of lubrication technology and impact protection structures.

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