Abstract
Tetraethylammonium tris[diethylthio-, di(n-butylthio)- or trimethylenedithio-tetrathiafulvalenyl(TTF)dithiolato] vanadium complexes (NEt 4 +1a,b,c - ) were oxidized with iodine to give the corresponding neutral complexes (1a,b,c), in which one unpaired electron is preferentially distributed at the TTFdithiolato groups. The compressed pellets of 1a,b,c exhibited comparatively low room-temperature electrical conductivities (σ RT 's) of 10 -(4-8) S cm -1 , which are however higher by 10 2-6 times than that (<10 -10 S cm -1 ) in a neutral bis(5,6-dihydro-1,4-dithiin-2,3-dithiolato) vanadium complex, V(DDDT) 3 .
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