Abstract
We utilized femtosecond time-resolved coherent anti-Stokes Raman spectroscopy (CARS) to study the ultrafast vibrational dynamics in distilled water at room temperature. The CARS signals from the broad OH-stretching modes between 3100cm−1 and 3700cm−1 were obtained and analyzed. The dephasing times of four Raman modes in water were detected and compared.
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