Abstract
Femtosecond time-resolved coherent anti-Stokes Raman spectroscopy (CARS) is utilized to study the ultrafast vibrational dynamics in ethanol at room temperature. The beat wavenumbers between Raman modes of CH stretch modes (from 2800cm−1 to 3000cm−1) in ethanol are excited and detected by varying wavelengths of the laser pulses and detection window. The coherence relaxation times of the CH stretch mode in ethanol are measured.
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