Abstract
Abstract The experimental vibrational frequencies for C(CN)4 from literature were re-assigned with the aid of approximate force field calculations. Refined force fields were deduced on the basis of (I) the original experimental assignment and (II) the present re-assignment. Calculated mean amplitudes of vibration and Bastiansen-Morino shrinkage effects strongly support the re-assignment (II) when comparing with gas electron diffraction results.
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