Abstract
A model of the dense disordered state, pertinent to chain and small molecule fluids is discussed. It rests on a quasi-lattice or cell model, with additional configurational disorder provided by vacancies. In the theory two parameters define the intermolecular interactions. In polyatomic systems a third parameter ensues, quantifying molecular modes of motion (i.e. soft vibrations and rotations) which are perturbed by the surroundings. In mixtures these parameters are explicit functions of composition and of self and cross interactions.
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