Model for coupled 4f−3d magnetic spectra: A neutron scattering study of the Yb-Fe hybridization in Yb3Fe5O12

Abstract

In this work, we explore experimentally and theoretically the spectrum of magnetic excitations of the Fe$^{3+}$ and Yb$^{3+}$ ions in ytterbium iron garnet (Yb$_3$Fe$_5$O$_{12}$). We present a complete description of the crystal-field splitting of the $4f$ states of Yb$^{3+}$, including the effect of the exchange field generated by the magnetically ordered Fe subsystem. We also consider a further effect of the Fe-Yb exchange interaction, which is to hybridise the Yb crystal field excitations with the Fe spin-wave modes at positions in the Brillouin zone where the two types of excitations cross. We present detailed measurements of these hybridised excitations, and propose a framework which can be used in the quantitative analysis of the coupled spectra in terms of the anisotropic $4f-3d$ exchange interaction.