Measurements of natural radioactivity and evaluation of radiation hazard indices in soils around the Manyoni uranium deposit in Tanzania

Abstract

Pre-mining natural radioactivity levels in soils over a 27.96 km2 site around the Manyoni Uranium Project in Tanzania were determined by a high purity germanium detector. The mean activity concentrations of 226Ra, 232Th, and 40K in soils were 227.43 ± 38.79 Bq/kg, 65.22 ± 3.70 Bq/kg, and 107.32 ± 23.07 Bq/kg, respectively. The average radium equivalent activity (Raeq), external hazard index (Hex), and internal hazard index (Hin) at these concentrations were 328.95 Bq/kg, 0.89, and 1.50, respectively. The mean absorbed dose rate in air at 1 m above the ground (Da) was 148.94 nGy/h, and the mean outdoor annual effective dose (Ed) was 0.18 mSv/y. Additionally, natural radioactivity levels in soils over a 0.71 km2 site, which is inside the 27.96 km2 site, which is prone to mine dust pollution above healthy levels, were also determined. The mean activity concentrations of 226Ra, 232Th, and 40K in the soils from this site were 380.4 ± 59.93 Bq/kg, 78.69 ± 8.99 Bq/kg, and 70.40 ± 7.91 Bq/kg, respectively. The corresponding means for Raeq, Hex, and Hin were 498.35 Bq/kg, 1.35, and 2.37, respectively. The mean Da and Ed were 226.21 nGy/h and 0.28 mSv/y, respectively. The average values of Ed at both sites were less than the public exposure limit of 1 mSv/y. This means that the sites have normal background radiation levels that do not endanger people's health when they engage in outdoor activities. When mining begins, the natural radioactivity levels obtained in this study, rather than national or global averages, can be used by mine owners or government agencies to assess the environmental effects of mining. Even after mining and during decommissioning, these baseline levels can also be used to measure how well the land has been restored.