Abstract

We study theoretically the magneto-optical properties of suspensions of magnetic nanoparticles within liquid crystalline matrices whose structure has been explored using off-lattice canonical Monte Carlo simulations. We find, in particular, that such systems exhibit a very strong magnetic circular-dichroism signal generated by morphological transformations of the structural motives of magnetic nanoparticles. These occur when the liquid crystalline matrix passes from isotropic to nematic states upon application of an external magnetic field. Moreover, we find that such hybrid magnetic-nanoparticle/liquid-crystalline systems demonstrate strong Faraday effect in the visible regime.

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