Abstract
Lead‐free magnetoelectric (ME) laminated (80Bi0.5Na0.5TiO3‐20Bi0.5K0.5TiO3)/(Ni0.8Zn0.2)Fe2O4 (BNKT/NZFO) composites are prepared via a modified cofiring processing, combining grain refinement and liquid phase sintering with low sintering aid content. The microstructure, dielectric, ferroelectric, magnetic, and magnetoelectric properties are investigated by varying the thickness of NZFO layer. The results show that the coexistence of independent BNKT and NZFO phase and the presence of the morphotopic phase boundary in BNKT phase with high piezoelectric coefficient d33 of 131 pC/N are confirmed. Laminated composites have clear and well‐bonded interfaces across the two layers, as well as improved ME properties. The maximum ME voltage coefficient (αE31) of the laminated composite reach 115.1 mV cm−1 Oe−1 with an optimized BNKT/NZFO layer thickness ratio of 1/2. In addition, a zero‐biased ME response was observed in BNKT/NZFO laminated composites.
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