Abstract
The magnetic properties of the Co1-xFexCr2S4 solid solutions for compositions adjacent to CoCr2S4 were investigated using various techniques, including magnetization measurements and AC susceptibility. The results revealed that substituting Fe for Co in the CoCr2S4 compound led to changes in the magnetic behavior, such as the presence of ferrimagnetic ordering and the emergence of a cluster spin glass phase. The study found that the temperature of the ferrimagnetic transition (TC) decreased with increasing Fe concentration, indicating the influence of iron on the magnetic properties of the solid solutions. Additionally, the discovery of a cluster spin glass phase for specific compositions (x = 0, 0.1, 0.2, 0.4) suggests complex magnetic behavior in these materials. In summary, the study offers valuable insights into the magnetic properties of Co1-xFexCr2S4 solid solutions and highlights the potential for tuning their magnetic behavior through compositional variations.
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