Abstract

Magnetic exchange force microscopy (MExFM) is one of the most important methods to investigate the spin structure of magnetic surfaces. However, a deep understanding of the measured spin contrast and the spin-dependent forces is missing. For the prototypical antiferromagnetic MnO(001) and NiO(001) surfaces probed by ferromagnetic Fe tips we demonstrate by means of spin-polarized density functional theory that the differences in the tip-surface interaction are due to the distance-dependent occupation of the transition-metal $3d$ states. While agreement is achieved with recent MExFM measurements of NiO(001), we predict opposite spin-contrast for MnO(001).

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