Abstract

Liquid helium (LHe) at 4.2 K was electronically excited using a corona discharge for both negative and positive high voltages. The experiments were carried out for different pressures in the range from 0.1 to 10 MPa at constant temperature. The light emitted from the zone close to the tip was spectroscopically analyzed showing features from atoms and excimer helium. The shifts and widths of the observed lines and bands were found to depend on the applied hydrostatic pressure and on the tip polarity. Our analysis showed that classic pressure broadening theory cannot account for the observed widths and shifts rather than the presence of bubbles which surround single excited atoms and molecules. For positive tip polarities red shifted features distinct from pure He and He <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</sub> * were observed and tentatively assigned to "red satellites".

Highlights

  • LIQUID helium is a fascinating substance with many peculiarities due to its highly quantum nature

  • Our analysis showed that classic pressure broadening theory cannot account for the observed widths and shifts rather than the presence of bubbles which surround single excited atoms and molecules

  • A particular feature of liquid helium is its intense luminescence in the visible and near infrared spectral range. This luminescence has been observed from superfluid 4He bombarded with energetic electrons [1,2,3], from liquid helium excited by a corona discharge [4,5,6,7,8] as well as from 4He droplets excited by monochromatic synchrotron radiation [9,10,11]

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Summary

INTRODUCTION

LIQUID helium is a fascinating substance with many peculiarities due to its highly quantum nature. The mechanisms involved in such a discharge in the liquid phase are complicated and involve electronic avalanches, energy transfer, formation of shock waves and bubbles, etc Another complication is that the particle density in corona discharge is not uniform [18]: the region close to the tip has a high excitation density and resembles in many respects a plasma. We further show that additional red-shifted spectral features exist that cannot be explained by rotational line intensity distributions of thermalized excimer molecules. These features depend on the polarity of the corona discharge giving rise to a provisional assignment to 'red satellites' side-bands. The microscopic origin of these red satellites is presently unknown

EXPERIMENTAL TECHNIQUES
GENERAL REMARKS
SPECTRA FROM NEGATIVE CORONA DISCHARGES
SPECTRA FROM POSITIVE CORONA
DISCUSSION
RED SATELLITES IN NEGATIVE CORONA
RED SATELLITES IN POSITIVE CORONA
CONCLUSION

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