Abstract

The adiabatic T(H) curves measured in a Heisenberg pyrochlore Gd2Ti2O7 prove the existence of a macroscopic number of local soft modes in this compound. A spin gap of 25 GHz, developing in Gd2Ti2O7 on cooling down to 1.3 K (in the collective paramagneti phase), was observed by ESR spectroscopy. ESR of diamagnetically diluted crystals revealed the single-ion anisotropy energy to be about a quarter of Curie-Weiss temperature. This might be responsible for the observed energy gap. Below 1 K, in the magneticaly ordered phase, the pin excitations have a threebranch spectum with two enegy gaps

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