Long-term analysis of AOD separated by aerosol type in East Asia

Abstract

This study aimed to identify the temporal variations in aerosol loadings and sizes in East Asia based on a method that uses the linear particle depolarization ratio (δP) and coarse-mode fraction of volume concentration (CMFvc) from AERONET Sun/Sky radiometer data. East Asia is the polluted region. Pollution levels continue to increase as a result of population growth and increasing industrialization. The main pollution sources are derived from anthropogenic activities and Asian dust. The data were used to separate the total aerosol optical depths (τ) of mixed aerosol plumes into optical depths contributed by dust (τD), coarse- (τPC), and fine-mode pollution (τPF). We used data taken from 1999 to 2021 in East Asia (Beijing, Xianghe on the west, Seoul, Yonsei, Anmyon, and Gwangju in the middle, Osaka and Shirahama in the east, and Taipei in the south). We identified the regional differences; the contribution of τD and τPC to the total τ of Chinese sites was almost twice that of other East Asian sites. We analyzed the monthly, seasonal and annual values each of the three aerosol types contributed to total optical depth. The annual variations in τD and τPC from 1999 to 2021 showed a decreasing trend. In contrast, τPF either increased or became stagnant during that time. We conclude that aerosol types in East Asia may have changed. The Ångström exponent of fine-mode particles increased in most regions (0.0008–0.0103 yr−1 for the wavelength range 440–870 nm), which means the mean size of the fine-mode pollution particles tended to decrease, even though τPF increased. The change in particle size might be caused by the decrease in primary emission sources due to the strong air pollution reduction policies in China, Korea, and Japan. Therefore, we need to focus on the change in aerosol properties not just on aerosol loadings.