Abstract

This paper explores the potential of all-sky cameras to retrieve aerosol properties with GRASP code (Generalized Retrieval of Atmosphere and Surface Properties). To this end, normalized sky radiances (NSR) extracted from an all-sky camera at three effective wavelengths (467, 536 and 605 nm) are used in this study. NSR observations are a set of relative (uncalibrated) sky radiances in arbitrary units. NSR observations have been simulated for different aerosol loads and types with the forward radiative transfer module of GRASP, indicating that NSR observations contain information about the aerosol type as well as about the aerosol optical depth (AOD), at least for low and moderate aerosol loads. An additional sensitivity study with synthetic data has been carried out to quantify the theoretical accuracy and precision on the aerosol properties (AOD, size distribution parameters, etc.) retrieved by GRASP using NSR observations as input. As result, the theoretical accuracy on AOD is within ±0.02 for AOD values lower or equal than 0.4; while the theoretical precision goes from 0.01 to 0.05 when AOD at 467 nm varies from 0.1 to 0.5. NSR measurements recorded at Valladolid (Spain) with an all-sky camera for more than two years have been inverted with GRASP. The retrieved aerosol properties are compared with independent values provided by co-located AERONET (AErosol RObotic NETwork) measurements. AOD from both data sets correlate with determination coefficient (r2) values about 0.87. Finally, the novel multi-pixel approach of GRASP is applied to daily camera radiances together, by constraining the temporal variation in certain aerosol properties. This temporal linkage (multi-pixel approach) provides promising results, reducing the highly temporal variation in some aerosol properties retrieved with the standard (one by one or single-pixel) approach. This work implies an advance in the use of all-sky cameras for the retrieval of aerosol properties.

Highlights

  • Atmospheric aerosol particles, which are the solid and liquid particles floating in the atmosphere (Willeke et al, 1993), impact on the Earth’s radiative balance mainly through aerosol–radiation and aerosol–cloud interactions (Boucher et al, 2013)

  • In order to study the performance of the GRASP-CAM products using real measurements, the GRASP-CAM method has been applied to normalized sky radiances (NSRs) measurements obtained with the allsky camera at Valladolid

  • This paper has analysed in detail the feasibility of using normalized sky radiance (NSR) measurements at three effective wavelengths from an all-sky camera to retrieve aerosol properties using the GRASP code

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Summary

Introduction

Atmospheric aerosol particles (hereinafter, “aerosols”), which are the solid and liquid particles floating in the atmosphere (Willeke et al, 1993), impact on the Earth’s radiative balance mainly through aerosol–radiation and aerosol–cloud interactions (Boucher et al, 2013) These interactions are related to the direct absorption and scattering of incoming solar radiation, as well as the modification of cloud properties, like cloud lifetime and albedo, since aerosols act as water droplet or ice crystal nuclei. These interactions depend significantly on the aerosol load and properties like the aerosol size distribution, chemical composition or refractive index. Aerosol property monitoring on a global scale is a crucial task

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