Abstract
Experimental tie-line data were investigated for two quaternary systems of water + n-hexane + diethyl carbonate + dimethyl carbonate and water + toluene + isooctane + dimethyl carbonate, and two related ternary systems of water + n-hexane + diethyl carbonate and water + n-hexane + dimethyl carbonate at 298.15 K and ambient pressure. The experimental tie-line data have been correlated using a modified UNIQUAC model and an extended UNIQUAC model, both with multicomponent interaction parameters in addition to the binary ones.
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