Laser-induced indirect ignition of non-premixed turbulent shear layers

Abstract

This study uses direct numerical simulations to investigate the forced ignition of temporally-evolving turbulent subsonic shear layers separating a gaseous stream of methane (CH4) and a stagnant gas environment of molecular oxygen (O2). Ignition is forced by a thermal-energy source that heats up a small volume of gas during periods of time much shorter than the characteristic acoustic time scale. The kernel, including its initial rounded conical shape, resembles experimental observations after optical breakdown is achieved in a gas irradiated by a focused laser. Particular emphasis is placed on ignition phenomena observed when the laser is focused on the O2 environment outside the turbulent shear layer, where the local composition is far beyond the lean flammability limit. This represents an indirect mode of non-premixed ignition that develops after a relatively long period of time has passed since laser-energy deposition, when the eddies near the oxidizer edge of the turbulent shear layer are intercepted by a baroclinically-generated subsonic vortex of hot dissociated O2 ejected from the laser-energy deposition zone. The success of indirect ignition depends on the orientation of the laser beam, the thickness of the shear layer, and the kernel standoff distance from the oxidizer edge of the shear layer. An ignition Damköhler number is defined that accounts for these averaged effects in six different simulation cases. For near-unity ignition Damköhler numbers, the solution is also sensitive to the local instantaneous flow field prevailing near the oxidizer edge of the shear layer, in that a modification of the instantaneous pre-deposition flow field, while preserving its turbulence statistics, can produce different ignition outcomes.Novelty and significance statement This work investigates forced ignition in a canonical flow configuration – a non-premixed turbulent CH4/O2 shear layer – and analyzes mechanisms by which ignition can be unexpectedly achieved in adverse conditions. In particular, an ensuing laser-generated advection of hot dissociated gas is observed to ignite the shear layer even when the mixture at the laser focal point is not flammable, an observation first made in early experiments. This flow phenomenon, whose consequences on ignition of non-premixed turbulent flows have not previously been analyzed by direct numerical simulation, can significantly separate the laser-energy deposition zone from the ignition location and is linked to baroclinically generated vorticity due to the rounded conical shape of the energy kernel. The phenomenology analyzed here may impact the design of laser-based ignition systems for chemical propulsion.