Abstract
The photodissociation of vinyl fluoride in the presence of intense CO 2 TEA laser radiation is reported. Time resolved emission from vibrationally excited products as well as undissociated parent species reveal (1) the collisionless nature of the dissociation process, (2) that the main product channel is HF elimination, and (3) that the available energy of the transition state is preferentially channeled into HF vibration energy. Our results are compared to those of others where alternate methods of dissociation were employed.
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