Abstract
Summary The quasi-lattice treatment of ternary reciprocal systems of molten salts has been extended to quaternary systems of the type (A+, B+, C+, X−, Y−) dilute in A+ and X−. According to the model, the “apparent” association energy between A+ and X− in the mixed “solvent” BY+CY should be a non-linear function of the molar composition of the solvent, and a function of the temperature. The existing experimental data on ion association energies in mixed solvents appear to be insufficient to provide a conclusive test of these predictions.
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