Abstract
Metasurfaces offer compact routes to spatial and polarization control of luminescence from nearby emitters. The most common integration strategy is to coat a patterned metamaterial or metasurface with a film of light emitting material. For example, structures such as arrays of Au nanorods coated with achiral light emitters exhibit circularly polarized photoluminescence at specific outcoupled angles. However, the degree of circular polarization in these systems is limited to relatively low values, and does not coincide with the angles with high photoluminescence intensity.This talk will discuss an alternative strategy, where the light emitters are patterned instead. We show that this structure offers several advantages: rather than averaging over the contributions of emitters in many different locations, this system exhibits highly directional photoluminescence with high degrees of circular polarization. Most importantly, the photoluminescence intensity is high at the same angles where the degree of circular polarization is high.These patterned light-emitting nanostructures are formed using direct-write electron beam lithography on semiconductor nanocrystals. This versatile method is capable of forming structures with aspect ratios greater than 2 and feature sizes as small as 30 nm, photoluminescence is retained after patterning, and the system is robust to multiple patterning steps.
Published Version
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