Abstract
The first resonance hyper-Raman spectra of liquids are made possible using an intracavity scattering geometry in a synchronously pumped picosecond stilbene 420 dye laser. Comparisons are made with the corresponding UV resonance Raman spectra, which are generated by the second harmonic of the cavity dumped output. Information about both the vibrational and electronic states of sample molecules is obtained.
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