Abstract
The intermolecular contribution to spin relaxation by translational-rotational diffusion dynamics in molecular liquids is calculated for arbitrary relative time scales of the two stochastic processes. The resulting relaxation times are functions of variables that are proportional to ratios between rotational and translational diffusion constants, in substantial generalization of earlier theoretical approaches. In the first part the general treatment for symmetric-top molecules is given with a reduction to quadratures and a simpler version for the spherical case
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