Interface fracture of polymer films: blister test experiments and modelling

Abstract

The interface fracture between a rigid substrate and polymer film is investigated in this work using pressurised blister test experiments and modelling. The interface crack growth is studied for two different types of polymer films: stiff and compliant ones. The pressurised blister test is used to provide critical pressure-crack length curves for different loading media (water and electrolyte solutions) and loading rates. Two different analytical approaches and a numerical modelling concept are used to determine the critical total energy release rate as a function of the crack length (crack resistance curve or R-curve). A relatively flat R-curve is observed for the system with the stiff polymer film, whilst R-curve for the compliant film system exhibits an increasing tendency. The mixed-mode fracture behaviour occurs for both investigated polymer film systems, as shown by the value of the mixed-mode angle that is constant for all investigated crack lengths. R-curves are nearly unaffected by different loading media, whereas the loading rate has a strong influence on the interface fracture of the compliant file system. Finite element method-based prediction of the total energy release rate is in good agreement with that obtained from analytical expressions.