Abstract

Organic semiconductor microcavities forming strongly coupled exciton-polaritons are interesting systems due to their nonlinear coherent emission observed even at room temperature. Here, we investigate the incident angle and photon-energy-dependent photoemission from a planar organic microcavity to evaluate the relaxation efficiency towards the bottom of the lower polariton branch. We observe nonlinear increase in the vertical emission from the microcavity when the sample is pumped resonantly to the lower polariton branch with an incident angle of 30 to 55°. The observed results support the fast and efficient relaxation of organic microcavity polaritons within the lower polariton branch.

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