In-pile thermal conductivity of uranium dioxide at low burnup

Abstract

In-pile thermal conductivity of uranium dioxide (UO2) was investigated at low burnup levels (<0.2 kWd/kg-UO2) to elucidate the concurrent effects of the fission damage and the thermal recovery. In-pile experiments were performed in the Halden reactor. The fuel centerline and the cladding temperatures were measured during the experiments, and the power level of specially designed test rodlets were also monitored. The uncertainty of the pellet-cladding gap's thermal resistivity was minimized with a liquid-metal bond, while comparable measurements were made in reference test rodlets without liquid metal bonding. The experimental data were analyzed using the inverse heat transfer approach. The heat conduction equation was solved by applying the measured temperature of the cladding as a boundary condition, and the calculated fuel centerline temperature was compared with the measured fuel centerline temperature to determine the relative matrix resistivity. Results showed that the in-pile matrix resistivity, the phonon-lattice interaction terms of the thermal conductivity, was ∼1.5–2.5 times higher than its unirradiated value due to fission-induced damage. Furthermore, the in-pile annealing caused a significant recovery of the matrix resistivity, and the amount of recovery increased from ∼20 to ∼33%, while the annealing temperature increased from 700 to 1,000 °C.